Friday, January 11, 2019

quantum field theory - What is the orbital angular momentum (OAM) of individual photons?


Update @ 21.01.2018


People investigate and talk about orbital angular momentum (OAM) of photons. For example, see this well-cited paper here and the PRL here. The latter starts with the remark



It is well known that photons can carry both spin and orbital angular momentum (OAM).



By definition, a photon is a one-particle state with definite momentum and helicity. In quantum mechanics, the OAM doesn't commute with momentum, and therefore a momentum eigenstate is not an OAM eigenstate. By that logic, individual photons cannot have definite OAM. Does it mean that the situation changes in quantum field theory and particles with definite momentum can also have definite OAM?


Maggiore's book on Quantum Field Theory talks about the spin (or helicity, to be more precise) of photons by working out the action of the spin operator on one-particle photon states (see my answer here) brushing aside the action of OAM operator.





  • I'm eager to understand the quantum field theory perspective of the OAM of individual photons. What is the OAM of individual photons?




  • Is there some physical example that cannot be explained without assuming that individual photons carry nonzero OAM in addition to spin (or helicity, to be more precise)?





Answer



This is an interesting mix of misconceptions:




By definition, a photon is a one-particle state with definite momentum and helicity. In quantum mechanics, the OAM doesn't commute with momentum, and therefore a momentum eigenstate is not an OAM eigenstate. By that logic, individual photons cannot have definite OAM.



No, a correct definition of a photon doesn't need to assign it a definite momentum or helicity, or even a well-defined frequency. The most convenient basis expansions tend to have these properties, but that's not inherent to the definition of a photon.


The short of it is that when you quantize electromagnetism, you start off by finding a suitable basis of vector-valued functions $\mathbf f_n(\mathbf r)$ in which to expand the vector potential as $$ \mathbf A(\mathbf r,t) = \sum_n\bigg[a_n(t)\mathbf f_n(\mathbf r)+a_n(t)^*\mathbf f_n(\mathbf r)^*\bigg], $$ where $a_n(t)$ is the generalized coordinate corresponding to the mode $\mathbf f_n(\mathbf r)$, setting things up so that its Poisson bracket with its conjugate is $\{a_n,a_m^*\}=\delta_{mn}$, and then you quantize by replacing $a_n(t)$ with the annihilation operator of that mode, so that a state with a single photon on that mode is $a_n^\dagger|0⟩$.


Now, here's the important thing: there is no requirement that the mode functions $\mathbf f_n(\mathbf r)$ be plane-wave states with circular polarization. It's a convenient choice, but it's not the only possible choice. Photons are excitations of the classical mode in question. Thus, if the classical mode is a plane wave, the photon will have a well-defined linear momentum, but if it is e.g. a Laguerre-Gauss or a Bessel mode, it will have a well-defined orbital angular momentum.


And, exactly as with the basis mode functions themselves, a photon with well-defined angular momentum can be understood as a superposition of photons with well-defined linear momentum (and vice versa), in the same way that you can expand a plane wave in terms of Bessel functions and vice versa. More importantly, this extends to linear combinations of modes with different frequencies: these give single-photon wavepackets, which evolve in time and are not eigenstates of the field hamiltonian, but are still $N=1$ eigenstates of the photon-number operator and therefore equally valid as single-photon states as the single excitations of a monochromatic plane wave.




OK, thus far for the standard description of how to deal with orbital angular momentum within the larger framework of quantum electrodynamics and quantum field theory, or within the more restrictive subsets of those that are often called quantum optics. However, just because you can describe something in a quantum way doesn't mean that you need to, but unfortunately ruling out alternative possible explanations, as you ask in your second question,




Is there some physical example that cannot be explained without assuming that individual photons carry nonzero OAM in addition to spin (or helicity, to be more precise)?



is a rather hard proposition.


However, OAM in this respect is no different to any other degree of freedom of light, and for any experiment that requires photons and a quantum-mechanical description on a given coordinate, you can produce an working experiment built on OAM, from Mandel dips to Bell-inequality violations to quantum cryptography, for which a good review is



G. Molina-Terriza, J.P. Torres and L. Torner. Twisted photons. Nature Phys. 3, 305 (2007).



Now, if you want a direct mechanical detection of the angular momentum carried by a single-photon excitation of an OAM mode, then that's unlikely to be feasible - in the same way that it's likely to be infeasible for the linear momentum of that state, because both are very small and very hard to measure. In that respect, atomic absorption experiments showing modified selection rules are likely to be conceptually sufficient, but I'm unsure whether the experiment has been done as yet.




Finally, if you want a comprehensive yet readable introduction to the subject of the angular momentum of light, I would recommend




R.P. Cameron. On the angular momentum of light. PhD thesis, University of Glasgow (2014).



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