Saturday, July 13, 2019

nuclear physics - Why are pear-shaped nuclei possible?


In a recent question, Ben Crowell raised an observation which really puzzled me. I obtained a partial answer by looking in the literature, but I would like to know if it's on the right track, and a fuller explanation for it.


It is a well-known fact in atomic and molecular physics that electronic eigenstates of inversion-symmetric molecules never have electronic dipole moments. This is because the electromagnetic hamiltonian that governs molecular physics is parity invariant: under a reflection the eigenstates must map to themselves, but nonzero vector quantities - like dipole moments - must switch signs.


However, it was a fairly big news item earlier this year (see e.g. the University of York press release or the piece in Nature News, 8 May 2013) that atomic nuclei can be 'pear-shaped'. This was predicted in the fifties, such as e.g.




Stability of Pear-Shaped Nuclear Deformations. K. Lee and D. R. Inglis. Phys. Rev. 108 no. 3, pp. 774-778 (1957)



and was experimentally confirmed this year in



Studies of pear-shaped nuclei using accelerated radioactive beams. L. P. Gaffney, P. A. Butler et al. Nature 497, 199–204 (09 May 2013). E-print on L.P. Gaffney's L.U. page.



A pear-shaped nucleus is one that has a nonzero electric octupolar moment. The pear shape arises from the added contributions of quadrupole and octupole perturbations on a spherical shape, winding up with something like this:


enter image description here


However, this poses an immense problem, because octupole moments have odd parity. If you reflect a pear-shaped nucleus (as opposed to a rugby-ball-shaped quadrupolar one), you get a pear pointing the other way. Having such a nucleus requires a mixing of parity-even and -odd contributions to an energy eigenstate, and this is not allowed for eigenstates of the parity-conserving electromagnetic and strong interactions that (presumably) shape atomic nuclei.



To put this another way, having a pear-shaped nucleus requires a way to tell which way the pear will point. The nuclear angular momentum can break isotropy and provide a special axis, but the 'pear' is a vector (pointing from the base to the stem) and one needs parity-violating machinery to turn a pseudovector angular momentum into a vector quantity.


Another way to phrase this is by saying that if such an eigenstate were possible for a parity-conserving hamiltonian, then the reflected version should also be a degenerate, inseparable eigenstate. Having a unique such ground state means having a way to lift that degeneracy.


I can then pose my question: why are pear-shaped nuclei possible? Is my reasoning incorrect? That is, can parity-conserving hamiltonians lead to such parity-mixed eigenstates? Or are there in fact parity-violating interactions that decisively lift the degeneracies and shape these nuclei? If so, what are they?



Answer



I have a partial answer to my question, which I'm posting down here because the question was getting too long.


After a good look online at a bunch of confusing (to me) papers from the nuclear physics literature, I came upon this review:



Intrinsic reflection asymmetry in atomic nuclei. P. A. Butler and W. Nazarewicz. Rev. Mod. Phys. 68 no. 2, pp. 349-421 (1996).



Here they draw an analogy to the Jahn-Teller effect, which is originally a molecular physics principle that states that spatially degenerate ground states are in general not possible: there will always be some deformation of the molecule - or some other interaction, however small - that breaks the symmetry of the system and therefore necessarily lowers the energy of at least one of the degenerate states. Thus they explicitly state that




Stable reflection-asymmetric deformations in the body-fixed frame can be attributed to a parity-breaking odd-multipolarity interaction which couples intrinsic states of opposite parity.



Later on, they pinpoint the cause of this parity breaking to the weak interaction:



Parity violation (in the laboratory frame) is caused by the parity-nonconserving component, VPNC, of the weak interaction. The magnitude of this effect is of the order of αp=GFm2π/GS107, where GF is the Fermi constant and GS is the strong coupling constant.



If this is the case, my natural assumption is that a nucleus whose ground state is pear-shaped must be part of a nearly-degenerate doublet (which comes from the original degenerate ground state of the strong and electromagnetic interactions) separated by about 107 of the gap to the next excited state. The first, 'weakly' excited state would then also be pear-shaped, and would have the projection (pear shape vector)(angular momentum)

in the opposite direction to the ground state. Is this intuition correct?


No comments:

Post a Comment

classical mechanics - Moment of a force about a given axis (Torque) - Scalar or vectorial?

I am studying Statics and saw that: The moment of a force about a given axis (or Torque) is defined by the equation: $M_X = (\vec r \times \...