Is it true that the field strength $F_{\mu\nu}$ in a non-Abelian gauge theory with gauge group $G$ vanishes if, and only if, the gauge field $A_{\mu}$ is a pure gauge?
I can show one implication.
If $A_{\mu}=\frac{i}{g}U\partial_{\mu}U^{\dagger}$ where $U \in G$, then the field strength vanishes, but I am struggling with the other implication.
Answer
I) Vanishing field-strength $F=0$ does not imply that the gauge potential $A$ is pure gauge. It only holds locally. There could be global obstructions. In fact, topological obstructions could happen even if the gauge group $G$ is Abelian.
II) Let us sketched the proof of the local statement in a sufficiently small neighborhood $\Omega\subseteq M$ of a point $x_{0}\in M$.
For a point $x\in \Omega$ choose a path/curve $C$ from $x_0$ to $x$.
Define group element via a Wilson line $$\tag {1} U(x)~:=~P e^{\int_{C} \!A},$$ where $P$ denotes path ordering.
Next use the non-Abelian Stokes' theorem to argue that this definition (1) does not depend on the curve $C$, because $F=0$.
Finally, use the group-valued section (1) to gauge transform the gauge potential $A$ to be zero.
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